D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl...

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1 / 19 TENDL-2009β: Chasing JEFF-3.2 D. Rochman and A.J. Koning Nuclear Research and Consultancy Group, NRG, Petten, The Netherlands June 4, 2009

Transcript of D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl...

Page 1: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

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TENDL-2009β: Chasing JEFF-3.2

D. Rochman and A.J. Koning

Nuclear Research and Consultancy Group,

NRG, Petten, The Netherlands

June 4, 2009

Page 2: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Contents

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① Motivations:=⇒ a roadmap to consistent and state-of-the-art evaluations

② Concept:=⇒ Exp. Data + Resonances +TALYS + Monte Carlo =

TENDL-2009

③ Is TENDL-2009 available and when ?

④ Content 1:=⇒ Neutrons, protons, deuterons, tritons, alphas, photons

⑤ Content 2:=⇒ Neutrons: 19F to 281Ds (Z=110), from MF-1 to MF-34

⑥ Examples

⑦ Conclusions and Future Improvements

Page 3: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Concept: TALYS + Monte Carlo = TENDL-2009

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Experimentaldata (i.e. XS)

5000 randomENDF files

=⇒ TotalMonte Carlo

Compilations(EXFOR)

TALYS+MCPackage

AverageENDF file

TENDL-2009library

Adjustedparameters

Covariancefiles

Page 4: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Concept: Standard nuclear data scheme

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ResonanceParameters

Determ.Codes

ENDFGen. purp.

File NJOY MCNP

ExperimentalData

EXFOR TEFAL

Output

ENDF/EAFActiv.File

Proc.codes

FIS-PACT

NuclearModel

Parameters TALYSOtherCodes

-keff-Flux-Etc.

-Activation-Burn-up

Page 5: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Concept: Nuclear Data Scheme with covariances

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ResonanceParameters TARES

Determ.Codes

ENDFGen. purp.

File NJOY MCNP

ExperimentalData

EXFOR TEFAL

Output

ENDF/EAFActiv.File

Proc.codes

FIS-PACT

NuclearModel

Parameters TALYSOtherCodes

TASMAN

+ Covariances

+ Covariances

-keff-Flux-Etc.

+ Covariances

-Activation-Burn-up

+ Covariances

Monte Carlo: 1000 TALYS runs

Page 6: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Concept: Nuclear Data Scheme with Total Monte Carlo

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ResonanceParameters TARES

Determ.Codes

ENDFGen. purp.

File NJOY MCNP

ExperimentalData

EXFOR TEFAL

Output

ENDF/EAFActiv.File

Proc.codes

FIS-PACT

NuclearModel

Parameters TALYSOtherCodes

TASMAN TMC

+ Covariances

+ Covariances

-keff-Flux-Etc.

+ Covariances

-Activation-Burn-up

+ Covariances

Monte Carlo: 1000 runs of all codes

Page 7: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Is TENDL-2009 available ?

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Not yet, but...

www.talys.eu/tendl-2009beta

Her

e

Here

Here

Here

HereH

ere

Page 8: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Is TENDL-2009 available ?

7 / 19

Not yet, but...

www.talys.eu/tendl-2009beta

Her

e

Here

Here

Here

HereH

ere

Page 9: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Content 1- TENDL-2009

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� Neutrons: ENDF files, plots, ACE files

� Protons: ENDF files, ACE files

� Alphas: ENDF files, ACE files

� ...Ne

utron

Proto

n

Deute

ron

Trito

n

Alph

a

Heliu

m3

Photo

n

TENDL-2009 >1000 >1000 >1000 >1000 >1000 >1000 >1000TENDL-2008 348 344 336 339 342 338 327(JEFF-3.1) 381 26(ENDF/B-VII.0) 393 48 5 3 163

Page 10: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Content 2- TENDL-2009 Neutron library: 19F to 281Ds (t1/2 > 1 µsec)

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Default Calculations Medium Quality Better Quality

Nucl

ear

Charg

eZ

Mass A

0

8

16

24

32

40

48

56

64

72

80

88

96

104

112

120

0 13 26 39 52 65 78 91 104 117 130 143 156 169 182 195 208 221 234 247 260 273 286 299 312

TENDL-2009

JEFF-3.1 (shifted + 50 A)

Fe 46-66

Pb 180-241

Pu 229-247

Page 11: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Content 3- TENDL-2009 Transport, Activation and EAF files

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TENDL-2009

ENDF File (200 MeV)MF1-15, 32,33,34

Activation File (200 MeV)MF3,6, 33

EAF File (60 MeV)MF3, 33

Page 12: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Content 3- TENDL-2009 Transport, Activation and EAF files

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TENDL-2009

ENDF File (200 MeV)MF1-15, 32,33,34

Activation File (200 MeV)MF3,6, 33

EAF File (60 MeV)MF3, 33

E < 20 MeV all MTsE > 20 MeV MT5

E < 200 MeV all MTs

Page 13: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Content 4- TENDL-2009 Neutron library: from MF-1 to MF-34

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Content of a typical file up to 200 MeV (out of > 1000 files):

☞ MF-1: Description

☞ MF-2: Resonance parameters (Reich-Moore or Multi-level Breit Wigner)

☞ MF-3: Cross sections (n,tot), (n,el), (n,non), (n,inli), ..., (n,γ), (n,pi), (n,αi)

☞ MF-4: Elastic angular distribution (Legendre Polynomials)

☞ MF-6: Double differential distributions and spectra for (n,2n), ..., (n,αi)

☞ MF- 8-10: Isomeric cross sections

☞ MF-32: Resonance parameter covariances

☞ MF-33: Cross section covariances (with cross correlation)

☞ MF-34: Elastic angular distribution covariances (up to the 6th Legendrepolynomial coefficient)

Page 14: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Content 5- TENDL-2009: Actinides

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Element Isotopes Element IsotopesTh 208-227, 228-232, 233-239 Pa 213-230, 231,233, 234-239U 222-232, 233-238, 239-242 Np 225-236, 237, 238-244Pu 229-237, 238-244, 245-247 Am 232-238, 239-243, 245-247Cm 238-242, 243-248, 249-252 Bk 238-248, 249, 250, 251Cf 237-248, 249, 250-256 Es 241-253, 254, 255-257Fm 242-257 Md 245-260No...Ds

=⇒ 36 ”medium” or ”better” quality evaluations and 406 ”default” qualityevaluations (with isomers)

Page 15: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Examples 1: U-235

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TalysENDF/B-VII.0

40 Talys RandomExp235U(n,2n)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

2015105

2.0

1.5

1.0

0.5

0.0

This workENDF/B-VII.0

40 Talys RandomExp

235U(n,γ)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

10110010−110−2

100

10−1

10−2

10−3

10−4

TalysENDF/B-VII.0

40 Talys RandomExp

235U(n,inl)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

20151050

3.5

3.0

2.5

2.0

1.5

1.0

0.5

TalysJEFF-3.1

ENDF/B-VII.0Exp

235U(n,f)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

20151050

2.5

2.0

1.5

1.0

0.5

Page 16: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Examples 1: U-238

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TALYSENDF/B-VII.0

JEFF-3.1Exp238U(n,2n)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

2015105

2.0

1.5

1.0

0.5

0.0

TALYSENDF/B-VII.0

JEFF-3.1Exp

238U(n,γ)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

10110010−110−2

101

100

10−1

10−2

10−3

10−4

TALYSENDF/B-VII.0

JEFF-3.1

238U(n,inl)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

20151050

4

3

2

1

0

TALYSJEFF-3.1

ENDF/B-VII.0Exp 238U(n,f)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

20151050

1.5

1.0

0.5

Page 17: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Examples 2: Pu-241

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TalysENDF/B-VII.0

JEFF-3.1241Pu(n,2n)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

2015105

1.0

0.8

0.6

0.4

0.2

0.0

TalysENDF/B-VII.0

JEFF-3.1

241Pu(n,γ)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

10110010−110−2

101

100

10−1

10−2

10−3

10−4

TalysENDF/B-VII.0

JEFF-3.1

241Pu(n,inl)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

20151050

2.5

2.0

1.5

1.0

0.5

0.0

TalysJEFF-3.1

ENDF/B-VII.0Exp

241Pu(n,f)

Incident Energy (MeV)

Cro

ssse

ctio

n(b

)

20151050

3.0

2.5

2.0

1.5

1.0

0.5

0.0

Page 18: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Examples 3: Ga-69 and Ga-84

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∆σ/σ vs. E for 69Ga(n,γ)

10-3 10-1 101 103 105 1070

10

20

30

40

50

60

∆σ/σ

vs.

E fo

r 69

Ga(

n,γ)

10-3

10-1

101

103

105

107

0102030405060Li

near

Axe

s:

Rel

. Sta

ndar

d D

ev. (

%)

Loga

rithm

ic A

xes:

Ene

rgy

(eV

)

Cor

rela

tion

Mat

rix

0.0

0.2

0.4

0.6

0.8

1.0

0.0

-0.2

-0.4

-0.6

-0.8

-1.0

∆σ/σ vs. E for 84Ga(n,γ)

10-3 10-1 101 103 105 1070

10

20

30

40

50

60

∆σ/σ

vs.

E fo

r 84

Ga(

n,γ)

10-3

10-1

101

103

105

107

0102030405060Li

near

Axe

s:

Rel

. Sta

ndar

d D

ev. (

%)

Loga

rithm

ic A

xes:

Ene

rgy

(eV

)

Cor

rela

tion

Mat

rix

0.0

0.2

0.4

0.6

0.8

1.0

0.0

-0.2

-0.4

-0.6

-0.8

-1.0

Page 19: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Examples 4: 61−85Ga(n,inl)

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TENDL-2009

6162-63

66

64

65

68

67

7169

61−85Ga(n,inl)

Incident Neutron Energy (MeV)

Cro

ssSec

tion

(Bar

ns)

20151050

2.5

2.0

1.5

1.0

0.5

0.0

Page 20: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Examples 5: 60−85Ga(n,γ)

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TENDL-2009

6463

65-66

61

7268

60

60−85Ga(n,γ)

Incident Neutron Energy (MeV)

Cro

ssSec

tion

(Bar

ns)

10110010−110−210−3

100

10−1

10−2

10−3

10−4

Page 21: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Conclusions and Future improvements

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☞ - Consistent data files

☞ - Automatic updates

☞ - Extensive set of covariance files

☞ - Reproducible with TALYS-1.2 (released with the library and referencepapers)

☞ - Best TALYS and resonance parameters fitting

Release date: End of 2009 !

☛ - More adjustment to experimental data

☛ - More extensive validation

☛ - Addition of original URR

Page 22: D. Rochman and A.J. Koning · Fm 242-257 Md 245-260 No...Ds =) 36 flmediumfl or flbetterfl quality evaluations and 406 fldefaultfl quality evaluations (with isomers) Examples

Conclusions and Future improvements

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☞ - Consistent data files

☞ - Automatic updates

☞ - Extensive set of covariance files

☞ - Reproducible with TALYS-1.2 (released with the library and referencepapers)

☞ - Best TALYS and resonance parameters fitting

Release date: End of 2009 !

☛ - More adjustment to experimental data

☛ - More extensive validation

☛ - Addition of original URR