Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam...

25
Text optional: Institutsname Prof. Dr. Hans Mustermann www.fzd.de Mitglied der Leibniz-Gemeinschaft Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de E1 and M1 excitations in 54 Fe and low-energy M1 strength in open-shell Fe isotopes Ronald Schwengner Helmholtz-Zentrum Dresden-Rossendorf, 01328 Dresden, Germany

Transcript of Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam...

Page 1: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Text optional: Institutsname � Prof. Dr. Hans Mustermann � www.fzd.de � Mitglied der Leibniz-GemeinschaftRonald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

E1 and M1 excitations in 54Fe

and

low-energy M1 strength in open-shell Fe isotopes

Ronald Schwengner

Helmholtz-Zentrum Dresden-Rossendorf, 01328 Dresden, Germany

Page 2: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

The bremsstrahlung facility at the electron accelerator ELBE

Accelerator parameters:

• Maximum electron energy:

≈ 18 MeV

• Maximum average current:

≈ 0.8 mA

• Micro-pulse rate:

13 MHz

• Micro-pulse length:

≈ 5 ps

R.S. et al., NIM A 555, 211 (2005)

1 m

Be window

dipole

dipole

dipole

radiator

steerer

quadrupoles

quadrupole

electron-beam dump

quartz windowbeam

hardener

collimator

polarisationmonitor

target

PbPE

door

Pb

photon-beamdump

Pb

HPGe detector

experimentalcave

acceleratorhall

Page 3: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Detector setup at γELBE

Page 4: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

3γγγγ-ray beam parameters Values

Energy 1 – 100 MeV

Linear & circular polarization > 95%

Intensity with 5% ∆Eγ/Eγ > 107 γ/s

Electron Accelerator Facility180 MeV Linac pre-injector180 MeV – 1.2 GeV Booster Injector250 MeV – 1.2 GeV Storage RingFELs: planar (linear pol.) and helical (circular pol.)

For more details see:http://www.tunl.duke.edu/higs/

• Highest intensity (γ-rays/s/keV) γ-ray beam in the world

• Produces γ-rays by Compton backscattering inside the optical cavity of a storage-ring FEL

• Produces both linearly and circularly polarized beams

Courtesy of C. Howell (TUNL)

Page 5: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Flux spectra at γELBE and HIγS

4000 6000 8000 10000Eγ (keV)

0

100

200

300

400

Φγ (

(eV

s)−

1 )

γELBE HIγS

Photon flux

γELBE: bremsstrahlung

HIγS: quasimononergetic,

polarized γ beams

Page 6: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Measurements at γELBE and HIγS

10000 10500 11000Eγ (keV)

100

101

102

103

Cou

nts

HIγS

Ee = 13.9 MeV

γELBE

Eγ = 10.6 MeV

E1

M1

Identification of multipolarities

from scattering of polarized

γ radiation at HIγS.

E1 radiation in vertical detectors

and M1 radiation in horizontal

detectors.

Page 7: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Measurement at γELBE

0 2 4 6 8 10 12 14Eγ (MeV)

1

10

100

1000

I s (eV

b)

54Fe28 Energy-integrated scattering

cross sections of levels in 54Fe

(J = 1 assumed)

Page 8: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Measurements at γELBE and HIγS

6 7 8 9 10 11 12Eγ (MeV)

10−2

10−1

100

B(M

1) (

µ N

2 )

54Fe28

6 7 8 9 10 11 12Eγ (MeV)

10−4

10−3

10−2

B(E

1) (

e2 fm2 )

54Fe28

Transitions with clear M1 or E1 assignments from the experiments at HIγS.

Page 9: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Experimental and calculated B(M1) values in 54Fe

6 7 8 9 10 11 12 13Eγ (MeV)

10−3

10−2

10−1

100

B(M

1) (

µ N

2 )

54Fe28 1

+ 0

+

5 6 7 8 9 10 11 12 13Eγ (MeV)

10−3

10−2

10−1

100

B(M

1) (

µ N

2 )

54Fe28 1

+ 0

+EXP CALC

Calculations using NuShellX.

Page 10: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Experimental and calculated B(M1) values in 54Fe

6 7 8 9 10 11 12 13Eγ (MeV)

10−3

10−2

10−1

100

B(M

1) (

µ N

2 )

54Fe28 1

+ 0

+

5 6 7 8 9 10 11 12 13Eγ (MeV)

10−3

10−2

10−1

100

B(M

1) (

µ N

2 )

54Fe28 1

+ 0

+EXP CALC

Calculations by K. Sieja.

Page 11: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Low-energy enhancement in 54Fe28

0 1 2 3 4 5 6 7 8Eγ (MeV)

0

0.02

0.04

0.06

B(M

1) (

µ N

2 )

π = +

54Fe

56Fe

Values in 56Fe as in

PRL 113, 252502 (2014),

but without lower limits of B(M1)

and without gates in Ex .

Page 12: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Shell-model calculations of M1 strength functions

0 2 4 6 8 10 12 14 16Eγ (MeV)

10−1

100

101

102

103

f 1 (1

0−9 M

eV−

3 )

94Mo

(3He,

3He’) data

shell modelM1

E1 + M1(γ,n) data

E1

)-3

(M

eV

M1

f

-910

-810

-710

Fe, Voinov et al. (2004) 56

)γαHe,3

(

Fe, Larsen et al. (2013) 56

)γ (p,p'

SM calc

Fe56

(a)

(MeV)γE0 1 2 3 4 5 6 7

)-3

(M

eV

M1

f-9

10

-810

-710

Fe57

(b)Fe, Voinov et al. (2004)

57)γHe'

3He,

3 (

Fe, Larsen et al. (2013/2014) 57

)γ (p,p'

SM calc

RITSSCHIL NuShellX

R.S., S. Frauendorf, A.C. Larsen

PRL 111, 232504 (2013)

B.A. Brown, A.C. Larsen

PRL 113, 252502 (2014)

Page 13: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Shell-model calculations for 60Fe34,64Fe38,

68Fe42

Code: NuShellX@MSU[B.A. Brown and W.D.M. Rae, Nucl. Data Sheets 120, 115 (2014)]

Model space: CA48PN with CA48MH1 Hamiltonian (48Ca core)[M. Hjorth-Jensen, T.T.S. Kuo, and E. Osnes, Phys. Rep. 261, 125 (1995)]

Orbits: π(0f(6−t)7/2 , 0ft

5/2, 1pt3/2, 1p

t1/2) ν(0ff 5

5/2, 1pp3

3/2, 1pp1

1/2, 0gg9

9/2)

Limitations of occupation numbers:

- t = 0 to 2.- f 5 = 2 to 6.- p3 = 0 to 4 for 60Fe and 2 to 4 for 64,68Fe.- p1 = 0 to 2 for all.- g9 = 0 to 2, 4, 6 for 60,64,68Fe, respectively.

Calculations: 40 levels of each spin from 0 to 10 and of each parity.

Transition strengths: eπ = 1.5 e, eν = 0.5 e; gs = 0.9 g frees

Page 14: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

B(E2) values in Fe isotopes

Experimental and calculated reduced E2 transition strengthsof the 2+

1→ 0+

1transitions in 60,62,64,66,68Fe.

E (2+1) B(E2, 2+

1→ 0+

1) β2

(keV) (W.u.)EXP CALC EXP GLOB CALC CALC

60Fe34 824 772 13.6(14) 19.6 26.2 0.3162Fe36 877 544 14.7(18) 17.3 27.8 0.32

13.6(17)64Fe38 746 595 30.9+13.8

−7.2 19.1 26.8 0.3222.6(22)

66Fe40 574 568 21.0(21) 23.4 27.8 0.3268Fe42 522 616 24.2 25.4 0.31

Page 15: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Average M1 strengths in Fe isotopes

0 1 2 3 4 5 6Eγ (MeV)

0

0.02

0.04

0.06

B(M

1) (

µ N

2 )

π = +

64Fe

68Fe

60Fe

0 1 2 3 4 5 6Eγ (MeV)

0

0.02

0.04

0.06

0.08

B(M

1) (

µ N

2 )

π = −

64Fe

68Fe

60Fe

⇒ Enhancement of M1 strength toward very low transition energy.

⇒ Development of a bump around 3 MeV with increasing neutron number.

PRL 118, 092502 (2017)

Page 16: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Dipole strength functions in 151Sm and 153Sm

) -

3 S

F (

Me

8−10

7−10

6−10

Sm, present exp.151

(p,d)

, n ), FilipescuγSm(150

, n ), FilipescuγSm(152

), Kopecky, E1γSm(n,149

GDR

M1

nS

(MeV)γ

-ray energy Eγ0 2 4 6 8 10

) -

3 S

F (

MeV

γ

8−10

7−10

6−10

Sm, present exp.153

(p,d)

, n ), FilipescuγSm(152

, n ), FilipescuγSm(154

), Kopecky, E1γSm(n,149

GDR

M1

nS

(p,d) data:

A. Simon et al.

PRC 93, 034303 (2016)

⇒ First observation of upbend

and scissors resonance

in one nuclide

⇒ Strength in the scissors region

about twice of that found in

(γ, γ) experiments

Page 17: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Strength functions in 60Fe and 68Fe

0 1 2 3 4 5 6Eγ (MeV)

0

10

20

30

40

50

60

70f 1

(10−

9 MeV

−3 )

M1−60

Fe

M1−68

Fe

E1−RIPL

f 2 E

γ2 (10

−9 M

eV−

3 )

E2−60

Fe (x10)

E2−68

Fe (x10)

Dipole strength function

f1 = 16π/9 (hc)−3B(M1) ρ(Ex , J)

ρ(Ex , J) - level density

of the shell-model states,

includes π = +, π = −,

all spins from 0 to 10.

⇒ Strength in the scissors region

about three times that found in

(γ, γ) experiments.

PRL 118, 092502 (2017)

Eγ < 2 MeV 2 ≤ Eγ ≤ 5 MeV Sum60Fe34 5.67 3.52 9.1964Fe42 4.46 5.13 9.5968Fe42 3.98 6.63 10.61

B(M1)tot(µ2

N)

Page 18: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Absorption strength in 68Fe

0

0.2

0.4

0.6

0.8

1

B(M

1) (

µ N

2 )

68Fe

0+

gs 1+

0 1 2 3 4 5 6 7 8Eγ (MeV)

0

0.2

0.4

0.6

0.8

1

B(M

1) (

µ N

2 )

68Fe

0+

2 1+

0+

15

∑B(M1) (µ2

N) (2≤ Eγ ≤ 5 MeV)

0+1→ 1+ 0+

2→ 1+

60Fe34 0.66 1.9864Fe42 1.65 2.5968Fe42 1.74 3.45

⇒ Strength from excited statesabout two times that found in(γ, γ) experiments because ofmore strong M1 transitionsin the scissors region.

PRL 118, 092502 (2017)

Page 19: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

M1 transitions in 68Fe

0

1

2

3

4

5

6

0 1 2 3 4 5 6 7 8 9 10

Ex (

MeV

)

J

68Fe π = +

Transitions with B(M1) > 0.1µ2

N.

Line widths ∼ B(M1) values.

Ji = Jf , Jf ± 1, Eγ < 2 MeV:low-energy upbend

Ji = Jf ± 1, Eγ ≈ 3 MeV:scissors region

Ji = Jf + 1, Ex ∼ J(J + 1):shears bands

Page 20: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Nuclear rotation

electric (collective) rotation magnetic rotation

J

z

x

E2

M1

M1

M1

M1

M1

M1

M1

E2

E2

E2

E2

E2

M1

M1

M1

M1

M1

M1

E2

E2

E2

E2

B(E2) ∼ Q20 B(M1) ∼ µ2

E x =h2

2ΘJ(J + 1); E γ ∼ J

Page 21: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Predicted Appearance of magnetic rotation

0 20 40 60 80 100 120 140 160

0

20

40

60

80

100

120

140

Neutron Number N

ProtonNumberZ

j"

2

j

0.25

0.15

28 50

82

126

28

50

82

64

64

20

20

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Magnetic rotation - “Shears bands”

S. Frauendorf, Rev. Mod. Phys. 73, 463 (2001).

Examples at A ≈ 80:

H. Schnare et al., PRL 82, 4408 (1999).

R.S. et al., PRC 65, 044326 (2002).

R.S. et al., PRC 66, 024310 (2002).

R.S. et al., PRC 80, 044305 (2009).

Page 22: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

E2 transitions in 68Fe

0

5

10

0 1 2 3 4 5 6 7 8 9 10

Ex (

MeV

)

J

68Fe π = +

Line widths ∼ B(E2) values.

Ji = Jf , Jf ± 1:admixtures to dipole transitions

Ji = Jf + 2, Ex ≈ J(J + 1)/(2J ):collective bands

Page 23: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Average E2 strengths in 68Fe

0 1 2Eγ (MeV)

0

20

40

60

80

B(E

2) (

e2 fm4 )

68Fe, π = +

Ji = Jf + 2Ji = 2

34

5 6

7

810

9

Largest B(E2) valuesin rotational-like sequences:

Ex ≈ J(J + 1)/(2J )

Eγ ≈ (2J − 1)/J

J ≈ 12 MeV−1

Page 24: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Summary

◦ Photon-scattering experiments on 54Fe28 carried out at γELBE and HIγS. 30 prominent

E1 and 16 M1 transitions observed up to 11.5 MeV.

◦ Strength in the quasicontinuum in analysis. Additional experiment with bremsstrahlung

up to 7.5 MeV needed.

◦ Large-scale shell-model calculations performed for 60Fe34,64Fe38,

68Fe42.

Collective properties of yrast states are reproduced in the used model space.

◦ The low-energy M1 strength decreases with increasing neutron number and a bump in

the scissors region develops while the sum of the two stays nearly constant.

◦ The strength in the scissors region includes many transitions between excited states.

This explains the different strengths found in experiments using photoexcitation and

light-ion induced reactions.

Page 25: Fe 54 E1andM1excitationsin and low ... Schwengner | Institut für Strahlenphysik | γγγγ-ray beam parameters Values Energy 1 – 100 MeV Linear & circular polarization > 95% Intensity

Ronald Schwengner | Institut für Strahlenphysik | http://www.hzdr.de

Collaborators

Experiments at γELBE (HZDR): D. Bemmerer, R. Beyer, A.R. Junghans, T. Kogler,A. Wagner et al.

Experiments at HIγS (TUNL): M. Bhike, Krishichayan, W. Tornow,U. Gayer, H. Pai (U Darmstadt),V. Derya (U Koln)

Calculations: B.A. Brown (NSCL/MSU)S. Frauendorf (U Notre Dame)K. Sieja (IPHC/CNRS)