Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits...

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Electron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron spins as qubits 2. Quantum dot plans for single spin measurements 3. Clocking electrons on the surface of helium 4. Photoemission electron source

Transcript of Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits...

Page 1: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Electron Spin Qubits on Liquid Helium

Guillaume Sabouret and Stephen Lyon

Princeton University

1. Electron spins as qubits

2. Quantum dot plans for single spinmeasurements

3. Clocking electrons on the surface of helium

4. Photoemission electron source

Page 2: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Helium channels for electron transport• For storing and moving qubits, we need a fairly high qubit density

– electrons a few μm apart

• To electrostatically control individual electrons, the electrodesmust be no farther than a few μm from them

• The channels are a convenient way to produce helium films a fewμm deep, in a controlled manner

LHe

++-

-

-

• The electron motion iscontrolled with electrodesbelow the channels

• This is the structure of aburied-channel Si CCD

• Channel width and gateperiod = 4 μm; depth = 2 μm

Degenerate P+-Si

Page 3: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

• Can move qubits, so normally keep them far apart (dipole-dipole at 10μm ~ 104 sec)

• Residual spin-orbit interaction (v x E)– v ~ 106 cm/sec, E ~ 104 V/cm Beffective = B|| ~ 10-7 T

– B|| changes direction as electron scatters, so

– For ~ 100 nsec T2 ~ 106 sec

• 3He impurities on 4He surface (~ 0.01/μm2) with motional narrowing T2 ~ 105 sec

• Johnson noise currents in gate layers:

– d = distance to metal, t = metal film thickness– For degenerately-doped Si, d ~ 2μm, T ~ 30 mK T2 ~ 105 sec

– On thin helium (quantum dot & 2-qubit gate), degenerately-doped Si electrode, d ~400Å, t ~ 1000Å T2 ~ 1000 sec at 30mK

• Fluctuations of local spin density in nearby metal

– Thin helium, degenerately-doped Si electrode (p-type, T1 for holes ~30ps), d ~ 400Å,t ~ 1000Å T2 ~ 2000 sec at 30mK

• Nuclear spins in gates/channels (use degenerately boron-doped 28Si)– Free carriers rapidly relax nuclear spins > 104 sec

• Paramagnetic defects?

– Few defects with unpaired spins in Si, and those relaxed rapidly by free carriers

)coth(4

3

1)(64

20

20

220

kTkT

t

tddT

μ hh+

+=

220

2||

22

12

1/1

+= BT

Spin Decohence Times

Page 4: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

e- e-

+V

-V -V

Triplet

Singlet

h

d

Quantum dots to measure spins

LHe

0.0 0.1 0.2 0.3 0.4 0.5

0.0

0.1

0.2

0.3

0.4

0.5

0.6

0.7

Calculated Singlet-Triplet splitting

Post diameter: 0.24 mPost voltage: 1V

Helium thickness, h ( m)

0.5μm

1μm

Platinum post made with FIB

Diagram of a post and its harmonic potential

A post creates a harmonic potentialthat splits the singlet and triplet energylevels.

Page 5: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Planar quantum dot

R (nm)

0 50 100

Heig

ht (n

m)

0

80

+

-oxide

LHe

metal

Height

post planar

d2V/dr2 for post and planar dot, d=50nmand 1 volt bias (x100V/μm2)

Planar dot looks to be easier

to make than the post, and

should give ~2x larger levelspacing we’ll try this first

Page 6: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Spin Coherence - Measurement Plans(like in GaAs quantum dots)

or or

or or

or or

Initial State

TripletSinglet

Page 7: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Planar double quantum dot(Dipole-Dipole CNOT)

0

0

125

125

12.5 125

nm

nm

Page 8: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought tointeract with another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 9: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought tointeract with another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 10: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought tointeract with another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 11: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 12: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 13: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 14: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 15: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 16: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 17: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 18: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 19: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 20: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 21: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 22: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 23: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 24: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 25: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 26: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 27: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 28: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 29: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Illustration of Pixel Sequence

• An electron is taken out of memory, brought to interactwith another electron and is then read.

Memory registers

Interaction

Single Electron Transistor Gate

Post

(The surrounding white region ismore negative than any pixel, inorder to keep the electrons in the

channels)

...

Page 30: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Clocking Electrons on Helium

• How readily can we shift electrons around?

W. T. Sommer and D. J. Tanner,Physical Review Letters 27, 20 (1971).

- Measurement of the mobility of the electronsthat are free to move.

-These experiments do not tell us theefficiency with which we transfer electrons(CTE = charge transfer efficiency) – chargetrapping CTE 1.0

Many shifts# e

lectr

ons

pixels

CTE is normally seen as a smearingof a signal – start with manyelectrons on one gate and some getleft behind with each shift

Page 31: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Thick (~ 0.9 mm) helium device

Helium depth

~ 0.9 mm

Guard ring (negative) to

reduce interference from

electrons outside our gates

3mm wide

gates

1cm

long

Clock voltages

Electrons above gatesElectrons outside gates

Voltage induced on left

gate by the electrons

on the helium goes to

lockin amplifier

1 2 3 4 5 6

7

Picture of the actual device

1.55K

- All gates carry a common dc bias to hold electrons (+4V ~2.6x107 electrons/cm2 or 1 electrons per 4 m2)

Page 32: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

iii) To the left iv) Kick outi) To the right ii) Pause

1 7

t

e- e- e- e- e-

-4V

+4V

+7V

Clock Sequence

• We don’t have long shift register, so use sequence which kickselectrons off the He if they get “stuck” on a gate

– Clock electrons left and right but after transferring to gate 1 (left), raiseenergy on gates 6 & 7 (gates negative) to expel remaining electrons fromthe device

• Variable total period

(x3) (x3)

0V Top plate

Page 33: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

CTE Measurements

• At low frequency (7 Hz) findCTE = .999

• CTE decreases withincreasing frequency becauseelectrons must diffuse fromone pixel to another, andpixels are huge (3mm)

• CTE would be negligible in Sifor our pixel size and electrondensity

No evidence for strong electron trapping at low frequencies

Page 34: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Channel Device Fabrication

4 μm

Si and SiO2

layers areremoved

SiO2 0.25 μmp++ Si 1.25 μmSiO2 1 μmSi substrate

Gold gates aredeposited andFIB patterned

Indiumis deposited

The sample isflip-chip bonded toa sapphire substratecontaining thegold leads for the gates.

The intersticial spaceis filled with epoxy

The channelis patterned

Page 35: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Channel Device (~1.5μm)

View of the sample with the guard ring. (Thebumps arise from the strain of the flip-chipping)

Zoom on the channel. The 1.5 μm Silicon layeris open to reveal the underlying metallic gates.

12

34

56

7

120x10-6

100

80

60

40

20

0

Lockin

Sig

nal M

agnitude (

V)

300250200150100500

Time (s)

Lockin signal magnitude as a function of time. Making gatenumber 2 more negative interrupts the signal.

Gate 2 = -0.5V

Vhold = 2V, Vplane=1V, Vguard=-2V

Commercial HEMT at lowtemperature for readout

~100 e-

4 μm

Page 36: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Photoemission Source(Shyam Shankar)

• Problem with filaments: too much heat

• Wilen and Gianetta (1985)- Photoemission from Zinc- 1KW arc lamp focused into fiber

• Try low power lamp and small setup

Ground

+V

Fiber

Transparent

Zinc on

Sapphire

Liquid

Helium

Helium

film

Page 37: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Photoemission Source• Pulsed Xenon Source (Ocean

Optics PX-2)• 600 micron Solarization

resistant fiber• 10nm Ti / 20nm Zn on Sapphire

substrate• Get 107-108 electrons in about

20 seconds• Adjust charge up rate by

varying pulse rate

• Find threshold voltage of 2V(4V/cm)

Page 38: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

How do the Electrons get through theHelium film?

1. Emit overHelium

2. Tunnel throughHelium

3. Form a bubbleand then escape

Zn He Vacuum

Boil off Helium

1

Vacuum Level

Fermi Energy

Zn

Work Function

(4.3 eV)

1eV Barrier

UV Light

Helium Vacuum

2

3

– Get 200 times more current if no Helium present

– Only ~100nJ total energy in UV pulse – can’t boil film

No

Page 39: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Bubble States?

• Lamp flashes for 5μsevery 5ms (200 Hz)

• Low voltage (below 2Vthreshold) during lampflash and for a variabletime after flash

• Some electrons even afteralmost 1ms

s5μLamp

Flash

4V

1V

Applied

Voltage

Low Voltage Time

Page 40: Electron Spin Qubits on Liquid Heliumlyon/Paris Talks 2006/guillaume_04-06.pdfElectron Spin Qubits on Liquid Helium Guillaume Sabouret and Stephen Lyon Princeton University 1. Electron

Summary

• Developed a method to measure charge-transfer-efficiency on thick helium without building a longarray– Measured a of 0.999 at ~107 electrons/cm2 and low

frequency• CTE can be understood in terms of electron diffusion• No evidence of electron trapping• Cond-mat/0602228

• Demonstrated electron clocking in a 4 μm-widechannel

• Developed an electron photoemission source– Small, low power UV source– Photoemission mechanism not fully understood