1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en...

32
1 Liam P. Gaffney Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity Octupole collectivity studied using radioactive- studied using radioactive- ion beams ion beams 1

Transcript of 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en...

Page 1: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

1

Liam P GaffneyLiam P Gaffney

Oliver Lodge Laboratory University of Liverpool UKOliver Lodge Laboratory University of Liverpool UK

Instituut voor Kern- en Stralingsfysica KU Leuven Belgium Instituut voor Kern- en Stralingsfysica KU Leuven Belgium

Octupole collectivityOctupole collectivitystudied using radioactive-ion studied using radioactive-ion beamsbeams

1

2

Octupole Collectivity

λ = 2 Quadrupoleλ = 3 Octupole

68Se

90Se

144Ba

148150Nd

226Ra

Octupole correlations enhanced at magic numbers 34 56 88 134

Exotic regions of the Segreacute chart so far inaccessible

Radioactive Ion Beams are the key

Schiff momen

t

CP violationEDM

Odd-ATalk by Peter Butler earlier this morning

3

Octupole CollectivityMicroscopically

Intruder orbitals of opposite parity and ∆J ∆L = 3 close to the Fermi level

220Rn and 224Ra lie near Z=88 N=134

εF

20

28

50

82

126

184

34

56

88

134

4

Octupole CollectivityMacroscopically

Nuclei take on a ldquopearrdquo shape

Reflection asymmetric

bull β3-vibrationbull Static β3-deformationbull Rigid β3-deformation

Signatures

Odd-even staggering negative parity

Parity doublets in odd-A nuclei

Enhanced E1 transitions

Large E3 strength rarr =

5

Octupole Collectivity

Rn (Z=86)

Z = 34

Z = 56

Z = 88 N = 134

6

Radon-220 and Radium-224

220Rn 224Ra[ref] JFC Cocks et al Phys Rev Lett 78 (1997) and Nucl Phys A 645 (1999)

7

Coulomb Excitation

Projectile (Z1A1)

Target (Z2A2)

v

Sommerfeld parameter

ldquoSaferdquo Coulex

Reduced matrix elements

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 2: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

2

Octupole Collectivity

λ = 2 Quadrupoleλ = 3 Octupole

68Se

90Se

144Ba

148150Nd

226Ra

Octupole correlations enhanced at magic numbers 34 56 88 134

Exotic regions of the Segreacute chart so far inaccessible

Radioactive Ion Beams are the key

Schiff momen

t

CP violationEDM

Odd-ATalk by Peter Butler earlier this morning

3

Octupole CollectivityMicroscopically

Intruder orbitals of opposite parity and ∆J ∆L = 3 close to the Fermi level

220Rn and 224Ra lie near Z=88 N=134

εF

20

28

50

82

126

184

34

56

88

134

4

Octupole CollectivityMacroscopically

Nuclei take on a ldquopearrdquo shape

Reflection asymmetric

bull β3-vibrationbull Static β3-deformationbull Rigid β3-deformation

Signatures

Odd-even staggering negative parity

Parity doublets in odd-A nuclei

Enhanced E1 transitions

Large E3 strength rarr =

5

Octupole Collectivity

Rn (Z=86)

Z = 34

Z = 56

Z = 88 N = 134

6

Radon-220 and Radium-224

220Rn 224Ra[ref] JFC Cocks et al Phys Rev Lett 78 (1997) and Nucl Phys A 645 (1999)

7

Coulomb Excitation

Projectile (Z1A1)

Target (Z2A2)

v

Sommerfeld parameter

ldquoSaferdquo Coulex

Reduced matrix elements

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 3: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

3

Octupole CollectivityMicroscopically

Intruder orbitals of opposite parity and ∆J ∆L = 3 close to the Fermi level

220Rn and 224Ra lie near Z=88 N=134

εF

20

28

50

82

126

184

34

56

88

134

4

Octupole CollectivityMacroscopically

Nuclei take on a ldquopearrdquo shape

Reflection asymmetric

bull β3-vibrationbull Static β3-deformationbull Rigid β3-deformation

Signatures

Odd-even staggering negative parity

Parity doublets in odd-A nuclei

Enhanced E1 transitions

Large E3 strength rarr =

5

Octupole Collectivity

Rn (Z=86)

Z = 34

Z = 56

Z = 88 N = 134

6

Radon-220 and Radium-224

220Rn 224Ra[ref] JFC Cocks et al Phys Rev Lett 78 (1997) and Nucl Phys A 645 (1999)

7

Coulomb Excitation

Projectile (Z1A1)

Target (Z2A2)

v

Sommerfeld parameter

ldquoSaferdquo Coulex

Reduced matrix elements

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 4: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

4

Octupole CollectivityMacroscopically

Nuclei take on a ldquopearrdquo shape

Reflection asymmetric

bull β3-vibrationbull Static β3-deformationbull Rigid β3-deformation

Signatures

Odd-even staggering negative parity

Parity doublets in odd-A nuclei

Enhanced E1 transitions

Large E3 strength rarr =

5

Octupole Collectivity

Rn (Z=86)

Z = 34

Z = 56

Z = 88 N = 134

6

Radon-220 and Radium-224

220Rn 224Ra[ref] JFC Cocks et al Phys Rev Lett 78 (1997) and Nucl Phys A 645 (1999)

7

Coulomb Excitation

Projectile (Z1A1)

Target (Z2A2)

v

Sommerfeld parameter

ldquoSaferdquo Coulex

Reduced matrix elements

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 5: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

5

Octupole Collectivity

Rn (Z=86)

Z = 34

Z = 56

Z = 88 N = 134

6

Radon-220 and Radium-224

220Rn 224Ra[ref] JFC Cocks et al Phys Rev Lett 78 (1997) and Nucl Phys A 645 (1999)

7

Coulomb Excitation

Projectile (Z1A1)

Target (Z2A2)

v

Sommerfeld parameter

ldquoSaferdquo Coulex

Reduced matrix elements

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 6: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

6

Radon-220 and Radium-224

220Rn 224Ra[ref] JFC Cocks et al Phys Rev Lett 78 (1997) and Nucl Phys A 645 (1999)

7

Coulomb Excitation

Projectile (Z1A1)

Target (Z2A2)

v

Sommerfeld parameter

ldquoSaferdquo Coulex

Reduced matrix elements

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 7: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

7

Coulomb Excitation

Projectile (Z1A1)

Target (Z2A2)

v

Sommerfeld parameter

ldquoSaferdquo Coulex

Reduced matrix elements

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 8: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

8

REX-ISOLDEIsotopeSeparationOn-Line D-Etector

RIBE-Xperiment

RadioactiveIonBeam 14GeV protons

from PS BoosterA

Heated tungsten line (Ra)

Plasma ion source (Rn)

Ionised atoms diffuse out of target

B

Mass separationin HRS

C

DPost-acceleration

8 UCx

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 9: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

9

MINIBALL REX-ISOLDE

9

220Rn224Ra beam

~283AMeV

Coulex target~2mgcm2

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 10: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

10

MINIBALLbull Particle ID in a Double-Sided Si Strip Detector

bull Event by event Doppler correction

bull 17˚ lt θlab lt 54˚

bull Array of HPGe of 8 triple clusters

bull 6-fold segmentation for positioning

bull ε gt 7 for 13MeV γ-rays

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 11: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

11

Particle-gamma coincidences

Prompt Random

Normalisation = tprompt

trandom

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 12: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

12

Analysis - 224Ra NiSn

60Ni target - 21mgcm2

120Sn target - 20mgcm2

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 13: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

13

Analysis - 220Rn NiSn

60Ni target - 21mgcm2

120Sn target - 23mgcm2

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 14: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

14

Analysis - 220Rn γ-γ

γ(697 keV)

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 15: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

15

Analysis - 220Rn HighLow θ

High CoM θLow CoM θ

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 16: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

16

Analysis - 224Ra Gosia16 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 3- 5- 7- 2+γ)

-- 5

Delayed-coincidence[56] Lifetimes (2+ 4+) -- 2

CdSn high CoM range 239˚ lt θlab lt 403˚

γ-ray yield-- 8 + 7

Ni high CoM range 231˚ lt θlab lt 399˚

γ-ray yield-- 10

CdSn low CoM range 403˚ lt θlab lt 543˚

γ-ray yield-- 8 + 8

Ni low CoM range 393˚ lt θlab lt 532˚

γ-ray yield-- 7

Total 55 data points[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 055

16

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 17: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

17

Results - 224Ra

bull Consistent with rotational model

bull Unstretched E3 matrix elements are non-zero Rot-vib model predicts these vanish

bull Coupled with level energy data we observe a static octupole deformation in 224Ra Awai

ting p

ublicat

ion

Embar

goed b

y Jo

urnal

0+

2+

4+ 1-

3-

5-

3ℏ phonon

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
  • Slide 11
  • Slide 12
  • Slide 13
  • Slide 14
  • Slide 15
  • Slide 16
  • Slide 17
  • Slide 18
  • Slide 19
  • Slide 20
  • Slide 21
  • Slide 22
  • Slide 23
  • Slide 24
  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 18: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

18

Analysis - 220Rn Gosia15 free matrix elements + 6 normalisation factors

ldquoExperimentrdquo Number and type of data

Multi-nucleon transfer[12]

226Ra(58Ni60Ni)224Ra 232Th(136Xe128Te)224RaAlpha alpha-prime[3]

226Ra(ααrsquo2n)224RaAlpha(beta)-decay[4]

228Th(224Fr) rarr α(β)

Branching ratios (1- 5- 7-)

-- 3

Delayed-coincidence[56] Lifetimes (2+) -- 1

CdSnNi high CoM range 221˚ lt θlab lt 378˚

γ-ray yield-- 2 + 8 + 5

CdSnNi low CoM range 379˚ lt θlab lt 518˚

γ-ray yield-- 2 + 8 + 5

Total 34 data points

[1] Poynter et al Phys Lett B 232 447 (1989)[2] JFC Cocks et al Nucl Phys A 645 61 (1999)[3] Marten-Toumllle et al Z Phys A 336 27 (1990)[4] W Kurcewicz et al Nucl Phys A 289 (1977)[5] WR Neal and HW Kraner Phys Rev 137 B1164 (1965)[6] H Ton et al Nucl Phys A 155 235 (1970)

χ2 = 086

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
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  • Slide 32
Page 19: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

19

Results - 220Rn

bull Consistent with rotational model

bull No information on unstretched E3

bull Larger data set required to determine if lt1-||E3||2+gt or lt1-||E3||4+gt vanish

bull Not definitive determination of collective mode dynamic (vibrational) or static (rotational) from Q3 alone

bull δE and Δix implies a coupling of an octupole phonon to the even-spin rotational band

bull Magnitude of Q3 consistent with dynamic picture similar to Q3(208Pb) and Q3(232Th)

bull Dynamic collectivity in 220Rn

Awaiting publication

Embargoed by Journal

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
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Page 20: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

20

220Rn - Vibrational

QuickTimetrade and a decompressor

are needed to see this picture

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
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Page 21: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

21

Discussion and Interpretation

8 -8

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
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  • Slide 32
Page 22: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

22

Discussion and Interpretation

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
  • Slide 10
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  • Slide 27
  • Slide 28
  • Slide 29
  • Slide 30
  • Slide 31
  • Slide 32
Page 23: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

23

Comparison to theory

Q1

Q2

Q3

bull Cluster model [1] - Misses small Q1

- Q2 is consistently too low- Q3 trend not observed

bull Mean field HFB with D1S or D1M [2]- Predicts cancelation of Q1

- Differences in Q3 predictions

[1] Shneidman et al (2003) Phys Rev C 67(1) 14313

[2] Robledo L M amp Bertsch G F (2011) Phys Rev C 84(5) 54302

Awaiting publicationEmbargoed by Journal

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
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  • Slide 25
  • Slide 26
  • Slide 27
  • Slide 28
  • Slide 29
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  • Slide 31
  • Slide 32
Page 24: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

24

Summary amp Outlook

See talk by George OrsquoNeill at 1545 today

bull Demonstrated sensitivity and ability to measure E3 matrix elements with Radioactive Ion Beams (RIBs)

bull B(E3 3- -gt 0+) measured for the first time in Rn and only second measurement in Ra both to ~10 precision

bull Experimental values rule out trend of cluster models

bull Exposes detailed differences in parameterisations of mean field calculations

bull Proposal for measurements in 222226228Ra and Ba region

bull Odd-mass nuclei key to atomic EDM measurements

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
  • Slide 9
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  • Slide 32
Page 25: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

25

CollaboratorsTE Cocolios J Pakarinen JCederkall D Voulot F Wernander

Th Kroumlll S Boumlnig C Bauer M von SchmidB Bastin

T Grahn A HerzanA Blazhev M Seidlitz N Warr M Albers M Pfeiffer D Radeck

M Rudigier P ThoumlleP van Duppen N Bree J Diriken N Kesteloot

S Sambi K ReyndersL P Gaffney P A Butler M Scheck DT Joss SV Rigby

E KwanT Chupp

D Cline CY WuM Zielinska P Napiorkowski M Kowalczyk

DG JenkinsCERN-ISOLDE SwitzerlandTU Darmstadt GermanyGanil FranceUniversity of Jyvaumlskylauml FinlandUniversity of Koumlln Germany

KU Leuven Belgium

University of Liverpool UK Lawrence Livermore Laboratory USUniversity of Michigan USUniversity of Rochester USHIL University of Warsaw PolandUniversity of York UK

Thank youand the REX-ISOLDE and MINIBALL collaborations

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
  • Slide 8
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  • Slide 32
Page 26: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

26

Aside - Protons off

bull Evidence of rapid exponential decay in beam rate after protons cease

bull Comparison of direct production vs alpha decay of parent (T12 = 366 days)

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
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Page 27: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

27

Radon-220 and Radium-224

220Rn

224Ra

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
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Page 28: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

28

Simulation - 224Ra

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

  • Slide 1
  • Slide 2
  • Slide 3
  • Slide 4
  • Slide 5
  • Slide 6
  • Slide 7
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Page 29: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

29

Simulation - 224Ra

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

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Gosia Analysis

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Discussion and Interpretation - 224Ra

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Page 30: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

30

Gosia Analysis

Measured E2 matrix elements [efm2]

TransitionalDiagonal

Measured E3 matrix elements [efm3]

StretchedUn-stretched

[Ref] H J Wollersheim et al Nucl Phys A 556 261 (1993)

31

Gosia Analysis

32

Discussion and Interpretation - 224Ra

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Page 31: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

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Gosia Analysis

32

Discussion and Interpretation - 224Ra

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Page 32: 1 Liam P. Gaffney Oliver Lodge Laboratory, University of Liverpool, UK Instituut voor Kern- en Stralingsfysica, KU Leuven, Belgium Octupole collectivity.

32

Discussion and Interpretation - 224Ra

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